This review is aimed to inspire and facilitate the design of novel synthetic underwater adhesives, that will, in turn expand our understanding of the physical and chemical parameters that influence underwater adhesion. Finally, we discuss some potential applications of underwater adhesives and the current challenges in the field by using a tandem analysis of the reported chemical structures and their adhesive strength. We then present a detailed review of synthetic underwater adhesives that have been reported to date. Third, we explore the adhesive mechanisms showcased by mussels and sandcastle worms to overcome the challenges brought by water. Second, we describe the challenges brought by water when adhering underwater. In this review, we introduce the basic thermodynamics processes and kinetic parameters involved in adhesion. This review provides a comprehensive overview of the progress in the science of underwater adhesion over the past few decades. These naturally occurring adhesives have inspired the creation of several synthetic materials that can stick underwater – a task that was once thought to be “impossible”. Over the past few decades, the physicochemical examination of biological underwater adhesives has begun to decipher the mysteries behind underwater adhesion.
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